Oh I didn't know, it's true saves can turn out huge :)
I noticed something though. Vanilla simulations only have the level dat file, so I tried removing everything from zips except level dat and levelmetadata, and it seems to work just as well !
You save about 35 M that way! Notice that level.dat files are very compressed, like 16M zipped = 4M but png images are almost not compressed and are pretty big (because a complex png has almost zero redundant data). Some level-init dat were even bigger than level.dat, and apparently don't have any impact on simulations.
I'll test them later tonight when I'm back home, but the current size of the whole mod is 48.3 M after my savagery, if I confirm it doesn't remove important data.
I also noticed you kept some saves dependancies, so those could be removed by resaving.
Also, unrelated, would you be interested if rework the mod icon a bit? I've done a number of them that you can see here: https://mods.factorio.com/mod/MbrTestMod